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Chemical Reaction Engineeringx

Comparison of Diffusion Flux Models for Fischer-Tropsch Synthesis

A. Nanduri [1], P. L. Mills [1],
[1] Department of Chemical and Natural Gas Engineering, Texas A&M University - Kingsville, Kingsville, TX, USA

The Fischer-Tropsch Synthesis (FTS) is a highly exothermic condensation polymerization reaction of syngas (CO+H2) in the presence of Fe/Co/Ru-based catalysts to produce a wide range of paraffins, olefins and oxygenates, the latter of which is often called syncrude. Multi-Tubular Fixed ... Mehr lesen

A Wall-Cooled Fixed-Bed Reactor Model for Gas-Phase Fischer-Tropsch Synthesis

A. Nanduri [1], P. L. Mills [1],
[1] Department of Chemical and Natural Gas Engineering, Texas A&M University - Kingsville, Kingsville, TX, USA

In the early 1920’s, Gas-To-Liquids (GTL) and Coal-To-Liquids (CTL) technologies were developed to account for the depleting crude oil resources [1]. During this period, Franz Fischer and Hans Tropsch developed a process to convert synthesis gas (syn gas), derived from coal ... Mehr lesen

Development of a User Interface for Design of SO2 Oxidation Fixed-Bed Reactors

A. Nagaraj [1], P. L. Mills [1],
[1] Texas A&M University - Kingsville, Kingsville, TX, USA

H2SO4 is a very important chemical commodity, and indeed, a nation’s H2SO4 production has been a reasonably good indicator of its industrial strength for the last century or so1,2. Nearly 350 MM tons of H2SO4 was produced in 20143.The demand for H2SO4 in United States exceeds the supply ... Mehr lesen

Microscale Simulations of Catalyst Deactivation During Gas-Phase Upgrading of Biomass Pyrolysis Vapors

P. N. Ciesielski [1], D. Robichaud [2], B. Donohoe [1], M. Nimlos [2],
[1] Biosciences Center, National Renewable Energy Laboratory, Golden, CO, USA
[2] National Bioenergy Center, National Renewable Energy Laboratory, Golden, CO, USA

Catalytic fast pyrolysis is a process by which biomass may be converted into liquid hydrocarbon transportation fuels and chemical co-products that are alternative to their petroleum-derived counterparts. Chemical compounds in raw pyrolysis vapor have high oxygen content and therefore ... Mehr lesen

Modeling of Biocalcification in Non-Saturated Conditions

B. Courcelles [1], C. Raymond-Poirier [1],
[1] École Polytechnique de Montréal, Montréal, QC, Canada

In the context of increasing demographic pressures around the world, soil improvement techniques constitute viable alternatives to expensive foundations. Among these techniques, the biocalcification of granular soils appears as a promising alternative relying on the formation of calcium ... Mehr lesen

COMSOL Multiphysics® Simulation of Flow in a Radial Flow Fixed Bed Reactor (RFBR)

A. G. Dixon [1], D. S. Polcari [1], A. D. Stolo [1], M. Tomida [1],
[1] Department of Chemical Engineering, Worcester Polytechnic Institute, Worcester, MA, USA

For design of radial flow fixed bed reactors, it is important to ensure proper flow distribution through the catalyst bed. A 2D axisymmetric model of a radial-flow reactor was used to evaluate flow maldistribution through the catalyst bed and the pressure drop through the reactor for a ... Mehr lesen

Multi-Dimensional Adsorption Model of CO2/H2O Sorbent Bed

C. Gomez [1], R. F. Coker [1], J. Knox [1], G. Schunk [1]
[1] NASA MSFC, Huntsville, AL, USA

The primary interest of the VC (Vacuum Characterization) test is to experimentally characterize the adsorption and vacuum desorption of CO2 and water vapor of a pelletized sorbent bed in a large diameter column. The VC test article is shown in Figures 1 and 2. The aluminum canister is 3” ... Mehr lesen

Combining Multiphysics Modeling and Solution Thermodynamics Using M4Dlib, an External Library

T. Marin-Alvarado [1],
[1] M4Dynamics, Toronto, ON, Canada

An external library, M4Dlib [1], has been developed to solve multiphysics problems coupled to solution thermodynamics. This approach extends the local equilibrium concept[2] to multiphysics modeling by incorporating a full Gibbs energy minimization routine at each numerical node to ... Mehr lesen

Transport Phenomena in the Conversion of an Anaerobic Landfill into an Aerobic Landfill

H. Omar [1], S. Rohani [1],
[1] University of Western Ontario, London, ON, Canada

The world’s landfills are beginning to fill up due to the growing human population. Landfills require land and there will come a time when there will be no land to be used for landfills. A solution that is gaining attraction is the conversion of traditional “dry-tomb” landfills (used for ... Mehr lesen

Dynamic Simulation of Interface Shapes During Chemical Vapor Deposition

J. V. Jayaramakrishna[1], S. K. Thamida[1]
[1]National Institute of Technology Warangal, Warangal, Telangana, India

Chemical Vapor Deposition (CVD) finds application in many manufacturing processes of microelectronic devices and MEMS as a recent development. It is also useful for preparation of functionalized surfaces in microsensor kind of devices. The phenomena that is studied is deposition of a ... Mehr lesen

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